Reply to “Comment on ‘Origin of symmetry-forbidden high-order harmonic generation in the time-dependent Kohn-Sham formulation’”

نویسندگان

چکیده

In reply to the Comment by O. Neufeld et al. [Phys. Rev. A 105, 047101 (2022)], we argue that conclusions of Phys. 103, 043106 (2021) remain valid. We disprove claim unphysical even-order harmonics originate from convergence issues related reflections at boundary simulation box. By additional calculations, show such perturb high-order harmonic generation spectra oscillations with periods much smaller than distance between harmonics. also demonstrate argument Comment, in contrast our multielectron excitations argument, cannot explain why there are no one-electron systems. Moreover, put forward conclude time-dependent Kohn-Sham equations superior natural is not

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Time-dependent Kohn-Sham approach to quantum electrodynamics

We prove a generalization of the van Leeuwen theorem towards quantum electrodynamics, providing the formal foundations of a time-dependent Kohn-Sham construction for coupled quantized matter and electromagnetic fields. We circumvent the symmetry-causality problems associated with the action-functional approach to Kohn-Sham systems. We show that the effective external fourpotential and four-curr...

متن کامل

Propagators for the time-dependent Kohn-Sham equations.

In this paper we address the problem of the numerical integration of the time-dependent Schrodinger equation i partial differential (t)phi=Hphi. In particular, we are concerned with the important case where H is the self-consistent Kohn-Sham Hamiltonian that stems from time-dependent functional theory. As the Kohn-Sham potential depends parametrically on the time-dependent density, H is in gene...

متن کامل

High-order harmonic generation in fullerenes with icosahedral symmetry

We investigate high-order harmonic generation in a sequence of icosahedral fullerenes using the extension of the so-called three-step or Lewenstein model to the molecular case. The high harmonic spectra obtained at midinfrared wavelengths show modulations in the plateau region. These modulations are due to the coherent superposition of the contributions from the atomic centers in the molecule t...

متن کامل

Comment on "transition to the relativistic regime in high order harmonic generation".

Experiments and computer simulations on the generation of high order harmonics from steep plasma gradients using intense femtosecond laser pulses are presented. Qualitative changes in the harmonic emission take place when the intensities are increased above 10(19) W/cm2 and/or the plasma scale length is varied. Good agreement between experimental and calculated spectra makes it possible to clea...

متن کامل

Time-dependent density functional theory beyond Kohn-Sham Slater determinants.

When running time-dependent density functional theory (TDDFT) calculations for real-time simulations of non-equilibrium dynamics, the user has a choice of initial Kohn-Sham state, and typically a Slater determinant is used. We explore the impact of this choice on the exchange-correlation potential when the physical system begins in a 50 : 50 superposition of the ground and first-excited state o...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: Physical Review A

سال: 2022

ISSN: ['1538-4446', '1050-2947', '1094-1622']

DOI: https://doi.org/10.1103/physreva.105.047102